Worldwide isotope ratios of the Fukushima release and early-phase external dose reconstruction

Measurements of radionuclides (RNs) in air made worldwide following the Fukushima accident are quantitatively compared with air and soil measurements made in Japan. Isotopic ratios RN:(137)Cs of (131)I, (132)Te, (134,136)Cs, are correlated with distance from release. It is shown, for the first time, that both within Japan and globally, ratios RN:(137)Cs in air were relatively constant for primarily particle associated radionuclides ((134,136)Cs; (132)Te) but that (131)I shows much lower local (<80 km) isotope ratios in soils relative to (137)Cs. Derived isotope ratios are used to reconstruct external dose rate during the early phase post-accident. Model "blind" tests show more than 95% of predictions within a factor of two of measurements from 15 sites to the north, northwest and west of the power station. It is demonstrated that generic isotope ratios provide a sound basis for reconstruction of early-phase external dose rates in these most contaminated areas.